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A2O78 A MB8< 2> 871560=85 >A;>6=5=89 ?@>F5AA0 8 703@O7=5=8O 7>;>B>- 8 A5@51@>A>45@60I53> M;N0B0 <54LN 8 =8:5;5< F5;5A>>1@07=> ?@5420@8B5;L=> 45A>@18@>20BL 8E 87 0=8>=8B0. 5A>@1F8O [Ag(CN)2]-. 0: >B<5G5=> 2KH5, =081>;55 MDD5:B82=K< 45A>@15=B>< F80=8ABKE A>548=5=89 A5@51@0 O2;O5BAO A;01>:8A;K9 @0AB2>@ ", A>45@60I89 8-10 3/; " + 2-2,5 3/; !1 8;8 H2SO4. @8 2708<>459AB288 A A5@51@>< " >1@07C5B :0B8>= =K9 :><?;5:A A>AB020 Ag[SC(NH2)2l3> He C45@68205<K9 0=8>=8B>< 8 ?5@5E>4OI89 2 M;N8@CNI89 @0AB2>@ ?> @50:F88: RAg(CN)2+3SC(NH2)2+2HCl=RCl+Ag[SC(NH2)2]3Cl+2HCN. > ?@8=F8?C 8>==>3> >1<5=0 F80=8ABK5 0=8>=K A5@51@0 E>@>H> 45A>@18@CNBAO @0AB2>@0<8 75-225 3/; NH^SCN + 10-20 3/; NaOH ?> @50:F88: RAg(CN)2+SCN-=RSCN+[Ag(CN)2]-. > B><C 65 ?@8=F8?C F80=84K A5@51@0 4>AB0B>G=> ?>;=> 45A>@18@CNBAO @0AB2>@0<8: 0) 250 3/; NH^NO^; 1) 100 3/; NaCN; 2) 2 <5=LH59 AB5?5=8 - @0AB2>@>< 150-200 3/; NaCl. !5@51@> ?>GB8 =5 45A>@18@C5BAO @0AB2>@0<8 NaOH. 5A>@1F8O [Cu(CN)n]n-1. &80=8ABK5 0=8>=K <548 MDD5:B82=> 45A>@18@CNBAO A;01>:8A;K<8 @0AB2>@0<8 " B>9 65 :>=F5=B@0F88, GB> 8 4;O 7>;>B0, 0 B0:65 I5;>G=K< @0AB2>@>< @>40=8AB>3> 0<<>=8O A :>=F5=B@0F859 50-75 3/; NH4SCN + 10-20 3/; NaOH. %>@>H> 45A>@18@CNBAO 0=8>=K <548 @0AB2>@>< F80=8AB>3> =0B@8O A :>=F5=B@0F859 40 80 3/; NaCN + 0,1 3/; NaOH ?@8 B5<?5@0BC@5 50 60 ! ?> @50:F88 >1<5=0: 2R2Cu(CH)3+2SC-=2RCN+[Cu(CN)3]2- 0B8>==K5 3@C??K 0=8>=8B0 ?@8 MB>< =59B@0;87CNBAO 8>=0<8 F80=0. 72;5G5=85 <548 2 @0AB2>@ ?@8 @0AE>45 53> 4> 10 >1J5<>2 =0 1 >1J5< A<>;K A>AB02;O5B 70 90%. @8 >1@01>B:5 A<>;K, A>45@60I59 :><?;5:A=K5 F80=84K <548, @0AB2>@0<8 <8=5@0;L=KE :8A;>B (2%-=>9 A5@=>9 8;8 A>;O=>9 :8A;>B>9) ?@>8AE>48B @07;>65=85 :><?;5:A>2 ?> @50:F8O<: *2RCu(CN)2+H2SO4=*R2SO4+2CuCN+2HCN; *R2Cu(CN)3+H2SO4=*R2SO4+CuCN+2HCN; *2R3!u(!N)4 + 3H2SO4 = *3R2SO4 + 2CuCN + 6HCN .  @57C;LB0B5 @07;>65=8O :><?;5:A>2 >1@07C5BAO >A04>: ?@>AB>3> F80=840 <548 CuCN, :>B>@K9 >AB05BAO 2 A<>;5, 8, A;54>20B5;L=>, <54L =5 45A>@18@C5BAO. <5AB5 A B5< ?@>8AE>48B G0AB8G=0O @535=5@0F8O F80=840, 2K45;ONI53>AO 2 2845 A8=8;L=>9 :8A;>BK HCN. 535=5@8@C5BAO F80=84 87 8>=>2: [Cu(CN)2] -  50%; [!u(!N)3]2- - 66,6%; [Cu(CN)4]3- - 75,0%. ;O M;N8@>20=8O <548 =5>1E>48<> >:8A;8BL >A04>: F80=840 <548 A ?5@52>4>< >4=>20;5=B=>9 <548 2 D>@<C :0B8>=0 !u2+, =5 C45@68205<>3> 0=8>=8B>< 8 CE>4OI53> A @0AB2>@><. @8 8A?>;L7>20=88 2 :0G5AB25 >:8A;8B5;O Fe2(SO4)3 (l,3%) 2 @0AB2>@5 H2SO4 M;N8@>20=85 ?@>E>48B ?> @50:F88 @8 MB>< F80=84 @535=5@8@C5BAO ?>;=>ABLN.  A;CG05 ?@8<5=5=8O !l 2 :0G5AB25 >:8A;8B5;O A;54C5B 8A?>;L7>20BL FeCl3. "0:8< >1@07><, ?@8<5=5=85 @0AB2>@0 A5@=>9 8;8 A>;O=>9 :8A;>B A >:8A;8B5;5< ?>72>;O5B M;N8@>20BL <54L A >4=>2@5<5==>9 ?>;=>9 @535=5@0F859 F80=840, GB> A>>B25BAB2C5B 40==K< ..;0:A8=0 8 . >6CE>2>9, ?>;CG5==K< ?@8 @535=5@0F88 F80=8ABKE @0AB2>@>2. A04>: CuCN <>6=> 872;5GL 87 A<>;K B0:65 :@5?:8< (40 50 3/;) @0AB2>@>< NaCN.@><5 C?><O=CBKE @5035=B>2, 45A>@1F8O F80=8ABKE 0=8>=>2 <548 <>65B ?@>872>48BLAO @0AB2>@0<8 NaCl A :>=F5=B@0F859 150-175 3/; ?> @50:F88 >1<5=0. @>F5AA ?@>B5:05B MDD5:B82=55 ?@8 ?>2KH5=88 B5<?5@0BC@K 4> 50-60 !. 5A>@1F8O [Zn(CN)4]2-. &8=: E>@>H> M;N8@C5BAO A> A<>;K @07102;5==K<8 @0AB2>@0<8 H2SO4 c :>=F5=B@0F859 20 25 3/;. @8 MB>< F80=8ABK9 :><?;5:A F8=:0 @07;0305BAO, F8=: ?5@5E>48B 2 D>@<C :0B8>=0 Zn2+, =5 C45@68205<>3> 0=8>=8B><, F80=84 ?>;=>ABLN @535=5@8@C5BAO.  A;CG05 ?@8<5=5=8O !l =5>1E>48<> 8A?>;L7>20BL @07102;5==K5 @0AB2>@K A :>=F5=B@0F859 0,1 =. (3 5 3/;) !l, B0: :0: ?@8 :>=F5=B@0F88 0,5 =. !l 8 2KH5 F80=8ABK9 :><?;5:A ?5@5E>48B 2 E;>@8ABK9 :><?;5:A ZnCI42-, :>B>@K9 7045@68205BAO 0=8>=8B><: R2Zn(CN)4+4HCl=R2ZnCl4+4HCN.  MB>< A;CG05 F8=: 2K2>48BAO 87 A<>;K ?@8 ?>A;54CNI59 ?@><K2:5 55 2>4>9 2A;54AB285 @07;>65=8O 0=8>=0 ZnCI2 A >1@07>20=85< @0AB2>@8<>9 A>;8 ZnCI2, 2 :>B>@>9 F8=: =0E>48BAO 2 2845 :0B8>=0 Zn2+, =5 7045@68205<>3> 0=8>=8B><.  A;CG05 ?@8ACBAB28O 2 A<>;5 8>=>2 D5@@>F80=840 [Fe(CN)6]4- :0B8>=K F8=:0 2 :8A;>9 A@545 >1@07CNB A =8<8 >A04:8 Zn2Fe(CN)6 8 H2ZnFe(CN)6 :>B>@K5 >AB0NBAO 2 A<>;5. > MB>9 ?@8G8=5 AB5?5=L :8A;>B=>9 45A>@1F88 F8=:0 C<5=LH05BAO.&80=8ABK5 A>548=5=8O F8=:0 MDD5:B82=> M;N8@CNBAO @0AB2>@0<8 NaOH A :>=F5=B@0F859 40-50 3/;. @8 MB>< ?@>B5:0NB @50:F88: *R2Zn(CN)4+6NaOH=*2ROH+Na2Zn(OH)4+4NaCN; Zn2Fe(CN)6+4NaOH=2Zn(OH)2+Na4Fe(CN)6; Zn(OH)2+2NaOH=Na2Zn(OH)4; *4ROH+Na4Fe(CN)6=*R4Fe(CN)6+4NaOH. 1@07CNI89AO F8=:0B-8>= [Zn(OH)4]2- A8;L=> 384@0B8@>20= 8 ?5@5E>48B 2 2>4=CN D07C. >= D5@@>F80=840 [Fe(CN)6]4- G0AB8G=> <>65B A>@18@>20BLAO 0=8>=8B><. ><?;5:A=K9 F80=84 F8=:0 A;01> M;N8@C5BAO @0AB2>@0<8 @>40=8AB>3> 0<<>=8O 8 E;>@8AB>3> =0B@8O, => 4>102;5=85 : MB8< @0AB2>@0< NaOH 2 :>;8G5AB25 20 3/; @57:> ?>2KH05B 872;5G5=85 F8=:0 87 A<>;K. "5B@0F80=>F8=:0B-8>= CA?5H=> 45A>@18@C5BAO B0:65 @0AB2>@>< 250-400 3/; NH4NO3 + 10 3/; NH4OH. &80=8ABK5 @0AB2>@K =5 45A>@18@CNB A>548=5=8O F8=:0. 5A>@1F8O [Ni(CN)4] 2-. =8>=K [Ni(CN)4] 2-, :0: 8 0=8>=K <548, 0:B82=> 45A>@18@CNBAO A;01>:8A;K< @0AB2>@>< ", 0 B0:65 I5;>G=K< @0AB2>@>< NH4SCN.  ?>A;54=5< A;CG05 45A>@1F8O ?@>B5:05B ?> @50:F88 >1<5=0: *R2Ni(CN)4+2SCH-=*2RSCN+[Ni(CN)4]2- -DD5:B82=> M;N8@C5BAO =8:5;L @07102;5==K<8 @0AB2>@0<8 A5@=>9 (20-25 3/;) 8;8 A>;O=>9 (10-20 3/;) :8A;>BK ?> @50:F88: *R2Ni(CN)4+2H2SO4=*R2SO4+NiSO4+HCN. @>F5AA ?@>B5:05B A >1@07>20=85< :0B8>=0 Ni2+=5 7045@68205<>3> 0=8>=8B><, 8 ?>;=>9 @535=5@0F859 F80=840. 0AB2>@ NH4NO3c :>=F5=B@0F859 250 3/; 45A>@18@C5B =8:5;L G0AB8G=> (>:>;> 40%). 0AB2>@K NaCN, NaOH, NaCl ?@0:B8G5A:8 =5 45A>@18@CNB F80=8ABK9 =8:5;L. 5A>@1F8O D5@@>F80=84-8>=0 [Fe(CN)6]4-. $5@@>F80=84-8>= MDD5:B82=> 45A>@18@C5BAO A 0=8>=8B0 @0AB2>@0<8 NaCN A :>=F5=B@0F859 50-100 3/;, ;CGH5 ?@8 B5<?5@0BC@5 4> 50-60 !. @>F5AA ?@>B5:05B ?> @50:F88 8>==>3> >1<5=0: *R4Fe(CN)6+4NaCN=*4RCN+Na4Fe(CN)6. =8>= [Fe(CN)6]4-E>@>H> 45A>@18@C5BAO B0:65 @0AB2>@0<8 2 3 =. NaCl (120-180 3/;) A A>45@60=85< 0,25-0,5 =. NaOH (10-20 3/;), ;CGH5 ?@8 B5<?5@0BC@5 50 60 !, ?> @50:F88 >1<5=0 A 8>=>< !1-. >AB0B>G=> ?>;=> 0=8>= [Fe(CN)6]4-M;N8@C5BAO @0AB2>@0<8 NH4SCN A :>=F5=B@0F859 75-225 3/; A ?5@5E>4>< A<>;K 2 @>40=84-D>@<C RSCN. >A;5 A5@=>-:8A;>B=>9 >1@01>B:8 A<>;K 4;O 45A>@1F88 F8=:0, =8:5;O 8 F80=84-8>=0 8 45A>@1F88 7>;>B0, A5@51@0 8 <548 A;01>:8A;K< @0AB2>@>< " <>6=> M;N8@>20BL 65;57> 8 >AB0B:8 <548 @0AB2>@>< A>AB020: 160 3/; NH4NO3 +50 3/; NH4OH + 40 3/; NaOH ?@8 B5<?5@0BC@5 25 !. 0AE>4 M;N8@CNI53> @0AB2>@0  7 >1J5<>2 =0 1 >1J5< A<>;K. >A;5 >1@01>B:8 65;57> 2 A<>;5 =0E>48BAO 2 D>@<5 A>@18@>20==>3> D5@@>F80=84-8>=0 R2Fe(CN)6 8 2 2845 >A04:>2 A>;59 Ni2Fe(CN)6, Zn2Fe(CN)6 8 4@., =5 @0AB2>@8<KE 2 :8A;>9 A@545, <54L - 2 2845 >A04:0 ?@>AB>3> F80=840 CuCN. I5;>G=>9 A@545 A>;8 D5@@>F80=840 A BO65;K<8 <5B0;;0<8 @07;030NBAO A >1@07>20=85< >A04:0 384@>:A84>2 Zn()2 8 Ni()2 8 D5@@>F80=84-8>=0 [Fe(CN)6]4-.&80=84 <548 8 384@0BK >:A84>2 <5B0;;>2 @0AB2>@ONBAO 2 0<<80G=>< @0AB2>@5 ?> @50:F8O<: CuCN+NH4NO3+2NH4OH=Cu(NH3)2NO3+NH4CN+2H2O; Zn(OH)2+2NH4NO3+2NH4OH=Zn(NH3)4(NO3)2+4H2O; Ni(OH)2+2NH4NO3+3NH4OH=Ni(NH3)5(NO3)2+5H2O; 1@07CNI85AO :><?;5:A=K5 :0B8>=K <548, F8=:0 8 =8:5;O ?5@5E>4OB 2 M;N0B. $5@@>F80=84-8>= 45A>@18@C5BAO A> A<>;K 8>=>< N03- ?> @50:F88 >1<5=0: *R4Fe(CN)6+4NO3-=*4RNO3+[Fe(CN)6]4-. =8>= [Fe(CN)6]4-G0AB8G=> (4> 40%) M;N8@C5BAO @0AB2>@0<8 2 4 =. HNO, 8 <0;> M;N8@C5BAO @0AB2>@0<8 2SO4 8 NaOH. [2] 5A>@1F8O [Co(CN)4]2-. &80=8ABK9 0=8>= :>10;LB0 A>45@68BAO 2 =0AKI5==>< 0=8>=8B5 >1KG=> 2 <0;>< :>;8G5AB25 (=5 1>;55 1 <3/3), => 45A>@1F8O 53> 70B@C4=5=0. 081>;55 MDD5:B82=> [Co(CN)4]2-M;N8@C5BAO @0AB2>@>< 150-375 3/; NH4SCN, G0AB8G=> (4> 30-60%) - @0AB2>@0<8 225-250 3/; NH4NO3, 180 3/; NaCI + 20 3/; NaOH, 50-100 3/; NaCN. 5A>@1F8O :>10;LB0 2>7@0AB05B A ?>2KH5=85< B5<?5@0BC@K 4> 50-60 !. 5A>@1F8O F80=84-8>=0 CN-. &80=84-8>= @535=5@8@C5BAO @0AB2>@0<8 A5@=>9 8;8 A>;O=>9 :8A;>B A :>=F5=B@0F859 10 20 3/; ?> @50:F88: *2RCN+H2SO4=*R2SO4+2HCN. &80=8AB>2>4>@>4=0O :8A;>B0 HCN >B3>=O5BAO 87 7>;>B0, ?>3;>I05BAO @0AB2>@>< NaOH 8;8 !0()2 8 2 2845 F80=8AB>9 I5;>G8 NaCN 8;8 Ca(CN)2 2>72@0I05BAO 2 ?@>F5AA F80=8@>20=8O. &80=84-8>= CN- 45A>@18@C5BAO B0:65 @0AB2>@0<8 NH4SCN, NH4NO3, NaCI, NaOH 8 4@., 0=8>=K :>B>@KE 70<5I0NB 53> 2 A<>;5. 5A>@1F8O ?@8<5A=KE 0=8>=>2 S2O32- , SO32- , SiO32- 8 4@. 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[2] 0 @8A. 1. ?@82545=0 B5E=>;>38G5A:0O AE5<0 ?5@5@01>B:8 7>;>B>A>45@60I53> AK@LO  8A.1 "%'!/ !%   " "! ) !+ ,/ 1.3 ,  &!! +/ "  "'+% -."  "%'! !% 72;5G5=85 7>;>B0 87 :8A;>3> B8><>G528==>3> M;N0B0 O2;O5BAO 7025@H0NI59 >?5@0F859 ?5@5@01>B:8 ?@0:B8G5A:8 ;N1>3> B8?0 @C4, 5A;8 2 B5E=>;>38G5A:>9 AE5<5 1K;0 8A?>;L7>20=0 >?5@0F8O B8>:0@10<84=>3> 2KI5;0G820=8O 7>;>B0. 081>;55 ?>43>B>2;5==K< : ?@><KH;5==><C 8A?>;L7>20=8N ?@8 ?5@5@01>B:5 7>;>BKE @C4 B5E=>;>38G5A:>3> B8?0  O2;O5BAO B8>:010<84. 1 MDD5:B82=>AB8 40==>3> @0AB2>@8B5;O, 2 G0AB=>AB8, <>6=> AC48BL ?> @57C;LB0B0< M:A?5@8<5=B>2, ?@82545==KE 2 B01;. 1. KI5;0G820=85 7>;>B0 ?@>872>48;>AL 87 @C4=KE A<5A59, A>AB02;5==KE 87 7>;>B>A>45@60I53> :20@F0 (2 ?@>1K @C4K A A>45@60=85< u A>>B25BAB25==> @02=K< 12,9 8 2.3 3/B) 8 22>48<KE 2 =53> @07;8G=KE <8=5@0;L=KE 4>102>:.  :0G5AB25 ?>A;54=8E 8A?>;L7>20=K: 1>@=8B-E0;L:>78=>2K9 :>=F5=B@0B (A>45@60=85 !u 70, S 20 %), HBCD=>9 0=B8<>=8B (98 % Sb2S3), A<5AL @50;L30@0 8 0C@8?83<5=B0. 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